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Directed Growth of Metal‐Organic Frameworks and Their Derived Carbon‐Based Network for Efficient Electrocatalytic Oxygen Reduction

Zhenhua Li, Mingfei Shao, Lei Zhou, Ruikang Zhang, Cong Zhang, Min Wei, David G. Evans, Xue Duan

📄 Abstract

A honeycomb-like carbon-based network is obtained by in situ nucleation and directed growth of metal-organic framework (MOF) arrays on the surface of layered double hydroxide (LDH) nanoplatelets, followed by a subsequent pyrolysis process, which exhibits largely enhanced electrocatalytic ORR performances. A successful paradigm for the directed growth of highly oriented MOF arrays is demonstrated, with potential applications for energy storage and conversion.

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