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Enhanced mobility CsPbI 3 quantum dot arrays for record-efficiency, high-voltage photovoltaic cells

Erin M. Sanehira, Ashley R. Marshall, Jeffrey A. Christians, Steven P. Harvey, Peter N. Ciesielski, Lance M. Wheeler, Philip Schulz, Lih Y. Lin, Matthew C. Beard, Joseph M. Luther

📄 Abstract

deficit. We show that charge carrier mobility within perovskite QD films is dictated by the chemical conditions at the QD-QD junctions. The AX treatments provide a method for tuning the coupling between perovskite QDs, which is exploited for improved charge transport for fabricating high-quality QD films and devices. The AX treatments presented here double the film mobility, enabling increased photocurrent, and lead to a record certified QD solar cell efficiency of 13.43%.

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