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Inorganic Lead Halide Perovskite Single Crystals: Phase‐Selective Low‐Temperature Growth, Carrier Transport Properties, and Self‐Powered Photodetection

Makhsud I. Saidaminov, Md Azimul Haque, Jawaher Almutlaq, Smritakshi Phukan Sarmah, Xiaohe Miao, Raihana Begum, Ayan A. Zhumekenov, İbrahim Dursun, Namchul Cho, Banavoth Murali, Omar F. Mohammed, Tom Wu, Osman M. Bakr

📄 Abstract

A rapid, low-temperature, and solution-based route is developed for growing large-sized cesium lead halide perovskite single crystals under ambient conditions. An ultralow minority carrier concentration was measured in CsPbBr3 (≈108 holes per cm3, much lower than in any other lead halide perovskite and crystalline silicon), which enables to realize self-powered photodetectors with a high ON/OFF ratio (105).

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