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Single-Crystal MAPbI3 Perovskite Solar Cells Exceeding 21% Power Conversion Efficiency

Zhaolai Chen, Bekir Türedi, Abdullah Y. Alsalloum, Chen Yang, Xiaopeng Zheng, Issam Gereige, Ahmed AlSaggaf, Omar F. Mohammed, Osman M. Bakr

📄 Abstract

Abstract Twenty-micrometer-thick single-crystal methylammonium lead triiodide (MAPbI3) perovskite (as an absorber layer) grown on a charge-selective contact using a solution space-limited inverse-temperature crystal growth method yields solar cells with power conversion efficiencies reaching 21.09% and fill factors of up to 84.3%. These devices set a new record for perovskite single-crystal solar cells and open an avenue for achieving high fill factors in perovskite solar cells.

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